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Creating a reusable adhesive that can hold objects on a wall and can yet be easily removed without causing damage has been a goal for researchers in the adhesives community for many years. 

Shaping 3D objects from 2D sheets enables form and function in diverse areas from art to engineering. Here we introduce kuttsukigami, which exploits sheet-sheet adhesion to create structure. The technique allows thin sheets to be sculpted without requiring sharp folds, enabling structure in a broad range of materials for a versatile and reconfigurable thin-sheet engineering design scheme. Simple closed structures from cylindrical loops to complex shapes like the Möbius loop are constructed and modeled through the balance between deformation and adhesion. Importantly, the balance can be used to create experimental measurements of elasticity in complex morphologies. More practically, kuttsukigami is demonstrated to encapsulate objects from the kitchen to micro scales and to build on-demand logic gates through sticky electronic sheets for truly reusable, reconfigurable devices. 

If an adhesive is meant to be temporary, roughness often poses a challenge for design. An adhesive could be made soft so that it can deform and increase surface contact but a softer material will in general hold a smaller load. Bioinspired adhesives, made with numerous microscale posts, show promise as roughness tolerant adhesives but are complicated to fabricate. In this work, we show how thin polymer sheets, when crumpled into a roughly spherical shape, form a very simple and roughness tolerant adhesive system. We use micro and macro-scale experiments to measure adhesion forces between various substrates and crumpled polydimethylsiloxane sheets. We find the force-displacement curves resemble probe-tack experiments of traditional pressure sensitive adhesives and that moderate tensile forces are required to initiate interfacial failure. Notably, we see that sticky crumples often perform better on long wavelength roughness than they do on smooth substrates. In order to improve the peak pull-off forces, we create a sticky crumple from a thin sheet of a glassy polymer, polycarbonate, coated with an adhesive layer. This elasto-plastic sticky crumple achieves high pull-off forces even on the rough surface of a landscaping brick. 

Capillary origami takes advantage of the surface forces of a liquid drop to assemble thin film structures. After a structure is assembled, the drop then evaporates away. The transient nature of the liquid drop means that the creation of dry and stable structures is impossible. Work presented in this paper shows that adhesion is, in fact, a key tool that enables the creation of stable, complex, capillary assembled origami structures, rather than a problem to be avoided. Here, polydimethylsiloxane thin films were used in several simple experiments designed to identify the balance between substrate–film adhesion and film–film adhesion in the context of capillary assembly. We then demonstrate how directional adhesion can be used to direct film peeling in order to create non-trivial patterned folds after a fluid drop is deposited. A minimal complex structure, a “double-fold” was created to demonstrate how adhesion uniquely facilitates multiple-step capillary assembly. Finally, a familiar “origami airplane” was created with these methods, demonstrating that adhesion aided capillary origami can be used to assemble complex, functional structures. 

In this work, we revisit experimentally and theoretically the mechanics of a tape loop. Using primarily elastic materials (polydimethylsiloxane, PDMS, or polycarbonate, PC) and confocal microscopy, we monitor the shape as well as the applied forces during an entire cycle of compression and retraction of a half-loop compressed between parallel glass plates. We observe distinct differences in film shape during the cycle; points of equal applied force or equal plate separation differ in shape upon compression or retraction. To model the adhesion cycle in its entirety, we adapt the ‘Sticky Elastica’ of [T. J. W. Wagner et al., Soft Matter , 2013, 9 , 1025–1030] to the tape loop geometry, which allows a complete analytical description of both the force balance and the film shape. We show that under compression the system is generally not sensitive to interfacial interactions, whereas in the limit of large separation of the confining parallel plates during retraction the system is well described by the peel model. Ultimately, we apply this understanding to the measurement of the energy release rate of a wide range of different cross-linker ratio PDMS elastomer half-loops in contact with glass. Finally, we show how the model illuminates an incredibly simple adhesion measurement technique, which only requires a ruler to perform.